Police said the Thursday morning accident involved a Nissan, saloon car and bodaboda rider.
According to the Kipande Road junction traffic police officer Boscombe Boy, the driver of the Nissan was trying to overtake a bus it collided head-on with oncoming saloon car and hit a bodaboda rider.
He said the driver has since been nabbed and is being detained at Nairobi Central Police Station.
The four victims were admitted at Nairobi West West hospital for emergency treatment.
The two bodies were taken to Nairobi City hospital mortuary.
The latest development comes barely a day when two people lost their lives on the spot in a head-on collision involving two trailers along mombasa road.
The two trailers were heading to different directions when one of them suffered a tyre burst leading to a collision and eventually the two burst into flames.
The incident is still under police investigations.
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